23,811 research outputs found

    Interparticle interactions:Energy potentials, energy transfer, and nanoscale mechanical motion in response to optical radiation

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    In the interactions between particles of material with slightly different electronic levels, unusually large shifts in the pair potential can result from photoexcitation, and on subsequent electronic excitation transfer. To elicit these phenomena, it is necessary to understand the fundamental differences between a variety of optical properties deriving from dispersion interactions, and processes such as resonance energy transfer that occur under laser irradiance. This helps dispel some confusion in the recent literature. By developing and interpreting the theory at a deeper level, one can anticipate that in suitable systems, light absorption and energy transfer will be accompanied by significant displacements in interparticle separation, leading to nanoscale mechanical motion

    Equation of state for hard sphere fluids with and without Kac tails

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    In this note, we propose a simple derivation of the one dimensional hard rod equation of state, with and without a Kac tail (appended long range and weak potential). The case of hard spheres in higher dimension is also addressed and it is shown there that our arguments --which avoid any mathematical complication-- allow to recover the virial form of the equation of state in a direct way.Comment: pedagogical pape

    Generalized Clustering Conditions of Jack Polynomials at Negative Jack Parameter α\alpha

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    We present several conjectures on the behavior and clustering properties of Jack polynomials at \emph{negative} parameter α=k+1r1\alpha=-\frac{k+1}{r-1}, of partitions that violate the (k,r,N)(k,r,N) admissibility rule of Feigin \emph{et. al.} [\onlinecite{feigin2002}]. We find that "highest weight" Jack polynomials of specific partitions represent the minimum degree polynomials in NN variables that vanish when ss distinct clusters of k+1k+1 particles are formed, with ss and kk positive integers. Explicit counting formulas are conjectured. The generalized clustering conditions are useful in a forthcoming description of fractional quantum Hall quasiparticles.Comment: 12 page

    Properties of Non-Abelian Fractional Quantum Hall States at Filling ν=kr\nu=\frac{k}{r}

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    We compute the physical properties of non-Abelian Fractional Quantum Hall (FQH) states described by Jack polynomials at general filling ν=kr\nu=\frac{k}{r}. For r=2r=2, these states are identical to the ZkZ_k Read-Rezayi parafermions, whereas for r>2r>2 they represent new FQH states. The r=k+1r=k+1 states, multiplied by a Vandermonde determinant, are a non-Abelian alternative construction of states at fermionic filling 2/5,3/7,4/9...2/5, 3/7, 4/9.... We obtain the thermal Hall coefficient, the quantum dimensions, the electron scaling exponent, and show that the non-Abelian quasihole has a well-defined propagator falling off with the distance. The clustering properties of the Jack polynomials, provide a strong indication that the states with r>2r>2 can be obtained as correlators of fields of \emph{non-unitary} conformal field theories, but the CFT-FQH connection fails when invoked to compute physical properties such as thermal Hall coefficient or, more importantly, the quasihole propagator. The quasihole wavefuntion, when written as a coherent state representation of Jack polynomials, has an identical structure for \emph{all} non-Abelian states at filling ν=kr\nu=\frac{k}{r}.Comment: 2 figure

    Laser-controlled fluorescence in two-level systems

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    The ability to modify the character of fluorescent emission by a laser-controlled, optically nonlinear process has recently been shown theoretically feasible, and several possible applications have already been identified. In operation, a pulse of off-resonant probe laser beam, of sufficient intensity, is applied to a system exhibiting fluorescence, during the interval of excited- state decay following the initial excitation. The result is a rate of decay that can be controllably modified, the associated changes in fluorescence behavior affording new, chemically specific information. In this paper, a two-level emission model is employed in the further analysis of this all-optical process; the results should prove especially relevant to the analysis and imaging of physical systems employing fluorescent markers, these ranging from quantum dots to green fluorescence protein. Expressions are presented for the laser-controlled fluorescence anisotropy exhibited by samples in which the fluorophores are randomly oriented. It is also shown that, in systems with suitably configured electronic levels and symmetry properties, fluorescence emission can be produced from energy levels that would normally decay nonradiatively. © 2010 American Chemical Society

    How to measure the Bogoliubov quasiparticle amplitudes in a trapped condensate

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    We propose an experiment, based on two consecutive Bragg pulses, to measure the momentum distribution of quasiparticle excitations in a trapped Bose gas at low temperature. With the first pulse one generates a bunch of excitations carrying momentum qq, whose Doppler line is measured by the second pulse. We show that this experiment can provide direct access to the amplitudes uqu_{q} and vqv_{q} characterizing the Bogoliubov transformations from particles to quasiparticles. We simulate the behavior of the nonuniform gas by numerically solving the time dependent Gross-Pitaevskii equation.Comment: 12 pages, 4 figures include

    Sensitive imaging of electromagnetic fields with paramagnetic polar molecules

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    We propose a method for sensitive parallel detection of low-frequency electromagnetic fields based on the fine structure interactions in paramagnetic polar molecules. Compared to the recently implemented scheme employing ultracold 87^{87}Rb atoms [B{\"o}hi \textit{et al.}, Appl. Phys. Lett. \textbf{97}, 051101 (2010)], the technique based on molecules offers a 100-fold higher sensitivity, the possibility to measure both the electric and magnetic field components, and a probe of a wide range of frequencies from the dc limit to the THz regime

    A photonic basis for deriving nonlinear optical response

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    Nonlinear optics is generally first presented as an extension of conventional optics. Typically the subject is introduced with reference to a classical oscillatory electric polarization, accommodating correction terms that become significant at high intensities. The material parameters that quantify the extent of the nonlinear response are cast as coefficients in a power series - nonlinear optical susceptibilities signifying a propensity to generate optical harmonics, for example. Taking the subject to a deeper level requires a more detailed knowledge of the structure and properties of each nonlinear susceptibility tensor, the latter differing in form according to the process under investigation. Typically, the derivations involve intricate development based on time-dependent perturbation theory, assisted by recourse to a set of Feynman diagrams. This paper presents a more direct route to the required results, based on photonic rather than semiclassical principles, and offers a significantly clearer perspective on the photophysics underlying nonlinear optical response. The method, here illustrated by specific application to harmonic generation and down-conversion processes, is simple, intuitive and readily amenable for processes of arbitrary photonic order. © 2009 IOP Publishing Ltd
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